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孙培培教授课题组在ORGANIC LETTERS发表研究论文

发布时间:17-08-04 14:36:19 文章来源:1 浏览次数: [ 字号:


Photoredox Catalysis: Construction of Polyheterocycles via Alkoxycarbonylation/Addition/Cyclization Sequence
Li, XX (Li, Xuanxuan)[ 1 ] ; Fang, XX (Fang, Xinxin)[ 1 ] ; Zhuang, SY (Zhuang, Shengyi)[ 1 ] ; Liu, P (Liu, Ping)[ 1 ] ; Sun, PP (Sun, Peipei)[ 1 ]*(孙培培)

[ 1 ] Nanjing Normal Univ, Jiangsu Collaborat Innovat Ctr Biomed Funct Mat, Sch Chem & Mat Sci, Jiangsu Prov Key Lab Mat Cycle Proc & Pollut Cont, Nanjing 210023, Jiangsu, Peoples R China

ORGANIC LETTERS, 201707,19(13),3580-3583

A novel visible-light-induced cascade reaction for the preparation of ester-functionalized polyheterocycles was developed under metal-free conditions, which was initiated. by an intermolecular radical addition to, a carbon carbon double bond of N-arylacrylamide derivatives-using alkyl carbazate as the ester source followed by cyano-,mediated cyclization. The desired phenanthriciine derivative products were isolated in moderate to high yields with broad substrate 'scope.


文章链接:
http://pubs.acs.org/doi/abs/10.1021/acs.orglett.7b01553
 


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